Numerical Simulation on the Rainout-Removal of Sulfur Dioxide and Acidification of Precipitation from Stratiform Clouds
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Graphical Abstract
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Abstract
The rainout-removal of SO2 and the acidification of precipitation from stratiform clouds are simulated using a one-dimensional, time-dependent model, parameterized microphysically in which dissolution and dissociation of gaseous SO2 and H2O2, and oxidation reaction in aqueous phase are taken into account. The effects of dynamic fac-tors, including updraft flow and turbulent transport, and the concentration of gaseous SO2 and H2O2 being transported into the clouds on pH value of the precipitation, the conversion rate S(IV)-S (VI) and the wet deposition rate of SO2 are discussed.
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